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SHEKARGOFTAR, M. POSPÍŠIL, J. DUGÁČEK, J. WEITER, M. HOMOLA, T.
Original Title
Surface Property Tuning of Methylammonium Lead Iodide by Plasma for Use in Planar Perovskite Solar Cells
Type
journal article in Web of Science
Language
English
Original Abstract
The demand for cheap and green energy as a replacement for fossil fuels has never been greater, and perovskite solar cells (PSCs) are among the leading means of meeting it. The surface properties of metal halide perovskite layers play crucial roles in the performance and durability of such cells. Consequently, a wide range of engineering processes for surface modification of perovskite layers has been investigated and among them is atmospheric pressure plasma (APP). Nevertheless, knowledge of the interaction between plasma and perovskite layers is still far from complete. In this work, CH3NH3PbI3 films were subjected to APP generated by a portable plasma source. A detailed understanding of band energy after plasma treatment is crucial to the investigation of the behavior of the perovskite layer. This study demonstrates a remarkable shift in the valence and conduction bands of a perovskite layer after plasma treatment, while band gap energy remains relatively constant. We found that short plasma treatment of perovskite layers resulted in higher performance and stability of PSCs.
Keywords
halide perovskite; atmospheric plasma; surface treatment; photoluminescence; energy band tuning
Authors
SHEKARGOFTAR, M.; POSPÍŠIL, J.; DUGÁČEK, J.; WEITER, M.; HOMOLA, T.
Released
28. 7. 2020
Publisher
AMER CHEMICAL SOC
Location
WASHINGTON
ISBN
2470-1343
Periodical
ACS OMEGA
Year of study
5
Number
29
State
United States of America
Pages from
18384
Pages to
18390
Pages count
7
URL
https://pubs.acs.org/doi/10.1021/acsomega.0c02179
Full text in the Digital Library
http://hdl.handle.net/11012/201790
BibTex
@article{BUT164814, author="Masoud {Shekargoftar} and Jan {Pospíšil} and Ján {Dugáček} and Martin {Weiter} and Tomáš {Homola}", title="Surface Property Tuning of Methylammonium Lead Iodide by Plasma for Use in Planar Perovskite Solar Cells", journal="ACS OMEGA", year="2020", volume="5", number="29", pages="18384--18390", doi="10.1021/acsomega.0c02179", issn="2470-1343", url="https://pubs.acs.org/doi/10.1021/acsomega.0c02179" }