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BOUCHAL, P. DVOŘÁK, P. HRTOŇ, M. ROVENSKÁ, K. CHMELÍK, R. ŠIKOLA, T. BOUCHAL, Z.
Original Title
Single-Shot Aspect Ratio and Orientation Imaging of Nanoparticles
Type
journal article in Web of Science
Language
English
Original Abstract
Plasmonic nanoparticleswith surface plasmon resonance (SPR) andscattering response dependent on their geometry and surrounding environmentare predestinated to be used as optical probes for sensing and imaging.Optical microscopy is capable of observing nanoparticles in variousmedia, but their geometry remains hidden below the diffraction limit.Here, a wide-field optical imaging technique is demonstrated, restoringthe aspect ratio and orientation of individual nanoparticles via thepolarization anisotropy (PA) measurement of the scattered light. ThePA is mapped into a single nanoparticle image, formed by decomposingthe scattered light into longitudinal and transverse SPR modes andmanipulating their angular momentum. The wide-field images providethe aspect ratio and orientation of many deposited nanoparticles allowingtheir assessment in heterogeneous suspensions or time-resolved measurements.In calibration experiments, orientation measurement accuracy and excellentsensitivity to nanoparticles with specific aspect ratios are demonstrated.Subsequently, the method is deployed in the automatic shape-dependentcategorization of hundreds of nanoparticles in a heterogeneous mixture.The single-shot capability is demonstrated in the time-resolved imagingof the electrophoretic deposition process.
Keywords
polarization anisotropy; light angular momentum; optical vortices; surface plasmon resonance; dark-fieldmicroscopy
Authors
BOUCHAL, P.; DVOŘÁK, P.; HRTOŇ, M.; ROVENSKÁ, K.; CHMELÍK, R.; ŠIKOLA, T.; BOUCHAL, Z.
Released
17. 8. 2023
Publisher
American Chemical Society
Location
WASHINGTON
ISBN
2330-4022
Periodical
ACS Photonics
Year of study
10
Number
9
State
United States of America
Pages from
3331
Pages to
3341
Pages count
11
URL
https://pubs.acs.org/doi/full/10.1021/acsphotonics.3c00785
Full text in the Digital Library
http://hdl.handle.net/11012/245044
BibTex
@article{BUT184511, author="Petr {Bouchal} and Petr {Viewegh} and Martin {Hrtoň} and Katarína {Rovenská} and Radim {Chmelík} and Tomáš {Šikola} and Zdeněk {Bouchal}", title="Single-Shot Aspect Ratio and Orientation Imaging of Nanoparticles", journal="ACS Photonics", year="2023", volume="10", number="9", pages="3331--3341", doi="10.1021/acsphotonics.3c00785", issn="2330-4022", url="https://pubs.acs.org/doi/full/10.1021/acsphotonics.3c00785" }