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Saeidi, S. Najari, S. Fazlollahi, F. Nikoo, M.K. Sefidkon, F. Klemeš, J.J. Baxter, L.L.
Originální název
Mechanisms and kinetics of CO2 hydrogenation to value-added products: A detailed review on current status and future trends
Typ
článek v časopise ve Web of Science, Jimp
Jazyk
angličtina
Originální abstrakt
Global warming, fossil fuel depletion and energy security are driving scientists to investigate the mechanism of hydrocarbons production from CO2 hydrogenation. The need for more comprehensive understanding on mechanism of CO2 hydrogenation to hydrocarbons remains controversial because of the complex reaction mechanism and a large number of involved species. The micro mechanism of CO2 hydrogenation to hydrocarbons has been considered as a possible remedy to fulfill the requirements. This review comprehensively discusses two processes: reverse water gas shift (RWGS) and CO2 hydrogenation to hydrocarbons. The review includes reaction mechanisms and catalyst effects on yields and rates. In addition, the review outlines each of the Fischer-Tropsch (FT) micro mechanisms. The review infers some mechanisms from existing work and proposes a new mechanism that improves several predictions. These mechanisms form the design basis for optimal reactor design
Klíčová slova
Modified Fischer-Tropsch synthesis; Microkinetics; Micromechanism; Enolic mechanism; Carbide mechanism
Autoři
Saeidi, S.; Najari, S.; Fazlollahi, F.; Nikoo, M.K.; Sefidkon, F.; Klemeš, J.J.; Baxter, L.L.
Vydáno
1. 12. 2017
ISSN
1364-0321
Periodikum
RENEWABLE & SUSTAINABLE ENERGY REVIEWS
Číslo
80
Stát
Spojené státy americké
Strany od
1292
Strany do
1311
Strany počet
20
BibTex
@article{BUT145949, author="Saeidi, S. and Najari, S. and Fazlollahi, F. and Nikoo, M.K. and Sefidkon, F. and Klemeš, J.J. and Baxter, L.L.", title="Mechanisms and kinetics of CO2 hydrogenation to value-added products: A detailed review on current status and future trends", journal="RENEWABLE & SUSTAINABLE ENERGY REVIEWS", year="2017", number="80", pages="1292--1311", doi="10.1016/j.rser.2017.05.204", issn="1364-0321" }