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Weigang Ma, Yiwei Zhu, Mohsin Ali Marwat, Pengyuan Fan, Bing Xie, David Salamon, Zuo-Guang Ye and Haibo Zhang
Originální název
Enhanced energy-storage performance with excellent stability under low electric fields in BNT–ST relaxor ferroelectric ceramics
Typ
článek v časopise ve Scopus, Jsc
Jazyk
angličtina
Originální abstrakt
Relaxor ferroelectrics are promising candidates for pulsed power dielectric capacitor applications because of their excellent energy-storage properties. Different from most relaxor ferroelectrics whose energy-storage density was improved by increasing the breakdown strength and reducing the remanent polarization, in this study, anti-ferroelectric (AFE) AgNbO3 (AN) was used to partially substitute the relaxor ferroelectric 0.76Bi0.5Na0.5TiO3–0.24SrTiO3 (BNT–ST) of morphotropic phase boundary (MPB) composition to reduce the remanent polarization while maintaining large maximum polarization. In this way, a large recoverable energy-storage density (2.03 J cm−3) was obtained in the BNT–ST–5AN ceramics under lower electric field of 120 kV cm−1, which is superior to other lead-free energy-storage materials under similar electric fields. Moreover, excellent temperature (25–175 °C) and frequency (1–100 Hz) stabilities are achieved. This performance demonstrates that the BNT–ST–5AN ceramics form a promising class of dielectric capacitive material for high-temperature pulsed power capacitors with large energy-storage density.
Klíčová slova
energy-storage; relaxor ferroelectric; large polarization; morphotropic phase boundary (MPB); temperature stability
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Vydáno
1. 1. 2019
ISSN
2050-7534
Periodikum
Journal of Materials Chemistry C
Ročník
7
Číslo
2
Stát
Spojené království Velké Británie a Severního Irska
Strany od
281
Strany do
288
Strany počet
8
URL
https://pubs.rsc.org/en/Content/ArticleLanding/2018/TC/C8TC04447C#!divAbstract
BibTex
@article{BUT151910, author="David {Salamon}", title="Enhanced energy-storage performance with excellent stability under low electric fields in BNT–ST relaxor ferroelectric ceramics", journal="Journal of Materials Chemistry C", year="2019", volume="7", number="2", pages="281--288", doi="10.1039/C8TC04447C", issn="2050-7534", url="https://pubs.rsc.org/en/Content/ArticleLanding/2018/TC/C8TC04447C#!divAbstract" }