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Benter, S. Dubrovskii, VG. Bartmann, M. Campo, A. Zardo, I. Sistani, M. Stoger-Pollach, M. Lancaster, S. Detz, H. Lugstein, A.
Originální název
Quasi One-Dimensional Metal-Semiconductor Heterostructures
Typ
článek v časopise ve Web of Science, Jimp
Jazyk
angličtina
Originální abstrakt
The band offsets occurring at the abrupt heterointerfaces of suitable material combinations offer a powerful design tool for high performance or even new kinds of devices. Because of a large variety of applications for metal- semiconductor heterostructures and the promise of low-dimensional systems to present exceptional device characteristics, nanowire heterostructures gained particular interest over the past decade. However, compared to those achieved by mature two-dimensional processing techniques, quasi one-dimensional (1D) heterostructures often suffer from low interface and crystalline quality. For the GaAs-Au system, we demonstrate exemplarily a new approach to generate epitaxial and single crystalline metal-semiconductor nanowire heterostructures with atomically sharp interfaces using standard semiconductor processing techniques. Spatially resolved Raman measurements exclude any significant strain at the lattice mismatched metal-semiconductor heterojunction. On the basis of experimental results and simulation work, a novel self-assembled mechanism is demonstrated which yields one-step reconfiguration of a semiconductor-metal core-shell nanowire to a quasi 1D axially stacked heterostructure via flash lamp annealing. Transmission electron microscopy imaging and electrical characterization confirm the high interface quality resulting in the lowest Schottky barrier for the GaAs-Au system reported to date. Without limiting the generality, this novel approach will open up new opportunities in the syntheses of other metal-semiconductor nanowire heterostructures and thus facilitate the research of high-quality interfaces in metal-semiconductor nanocontacts.
Klíčová slova
Nanowire; GaAs; gold; metal-semiconductor heterostructure; quasi 1D contacts
Autoři
Benter, S.; Dubrovskii, VG.; Bartmann, M.; Campo, A.; Zardo, I. ; Sistani, M.; Stoger-Pollach, M.; Lancaster, S. ; Detz, H.; Lugstein, A.
Vydáno
1. 6. 2019
ISSN
1530-6992
Periodikum
Nano Letters
Ročník
19
Číslo
6
Stát
Spojené státy americké
Strany od
3892
Strany do
3897
Strany počet
URL
https://pubs.acs.org/doi/10.1021/acs.nanolett.9b01076
BibTex
@article{BUT159146, author="Benter, S. and Dubrovskii, VG. and Bartmann, M. and Campo, A. and Zardo, I. and Sistani, M. and Stoger-Pollach, M. and Lancaster, S. and Detz, H. and Lugstein, A.", title="Quasi One-Dimensional Metal-Semiconductor Heterostructures", journal="Nano Letters", year="2019", volume="19", number="6", pages="3892--3897", doi="10.1021/acs.nanolett.9b01076", issn="1530-6992", url="https://pubs.acs.org/doi/10.1021/acs.nanolett.9b01076" }