Detail publikace

Source contributions and mass loadings for chemicals of emerging concern: Chemometric application of pharmaco-signature in different aquatic systems

Jiang, Jheng-Jie Lee, Chon-Lin Brimblecombe, Peter Vydrova, Lucie Fang, Meng-Der

Originální název

Source contributions and mass loadings for chemicals of emerging concern: Chemometric application of pharmaco-signature in different aquatic systems

Typ

článek v časopise ve Web of Science, Jimp

Jazyk

angličtina

Originální abstrakt

To characterize the source contributions of chemicals of emerging concern (CECs) from different aquatic environments of Taiwan, we collected water samples from different aquatic systems, which were screened for 30 pharmaceuticals and illicit drugs. The total estimated mass loadings of CECs were 23.1 g/d in southern aquatic systems and 133 g/d in central aquatic systems. We developed an analytical framework combining pollutant fingerprinting, hierarchical cluster analysis (HCA), and principal component analysis with multiple linear regression (PCA-MLR) to infer the pharmaco-signature and source contributions of CECs. Based on this approach, we estimate source contributions of 62.2% for domestic inputs, 16.9% for antibiotics application, and 20.9% for drug abuse/medication in southern aquatic system, compared with 47.3% domestic, 35.1% antibiotic, and 17.6% drug abuse/medication inputs to central aquatic systems. The proposed pharmaco-signature method provides initial insights into the profile and source apportionment of CECs in complex aquatic systems, which are of importance for environmental management.

Klíčová slova

Source apportionment; Emerging contaminants; Fingerprinting; Mass loading; Risk quotient

Autoři

Jiang, Jheng-Jie; Lee, Chon-Lin; Brimblecombe, Peter; Vydrova, Lucie; Fang, Meng-Der

Vydáno

3. 1. 2016

Nakladatel

ELSEVIER SCI LTD

Místo

OXFORD

ISSN

0269-7491

Periodikum

ENVIRONMENTAL POLLUTION

Ročník

208

Číslo

1

Stát

Spojené království Velké Británie a Severního Irska

Strany od

79

Strany do

86

Strany počet

8

URL

https://www.sciencedirect.com/science/article/pii/S0269749115003322

BibTex

@article{BUT170226,
  author="Jiang, Jheng-Jie and Lee, Chon-Lin and Brimblecombe, Peter and Vydrova, Lucie and Fang, Meng-Der",
  title="Source contributions and mass loadings for chemicals of emerging concern: Chemometric application of pharmaco-signature in different aquatic systems",
  journal="ENVIRONMENTAL POLLUTION",
  year="2016",
  volume="208",
  number="1",
  pages="79--86",
  doi="10.1016/j.envpol.2015.06.039",
  issn="0269-7491",
  url="https://www.sciencedirect.com/science/article/pii/S0269749115003322"
}