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ZINKIEWITZ, M. WOZNIAK, T. KAZIMIERCZUK, T. KAPUSCINSKI, P. ORESZCZUK, K. GRZESZCZYK, M. BARTOŠ, M. NOGAJEWSKI, K. WATANABE, K. TANIGUCHI, T. FAUGERAS, C. KOSSACKI, P. POTEMSKI, M. BABINSKI, A. MOLAS, M.
Originální název
Excitonic Complexes in n-Doped WS2 Monolayer
Typ
článek v časopise ve Web of Science, Jimp
Jazyk
angličtina
Originální abstrakt
We investigate the origin of emission lines apparent in the low-temperature photoluminescence spectra of n-doped WS2 monolayer embedded in hexagonal BN layers using external magnetic fields and first-principles calculations. Apart from the neutral A exciton line, all observed emission lines are related to the negatively charged excitons. Consequently, we identify emissions due to both the bright singlet and triplet) and dark (spin- and momentum-forbidden) negative trions as well as the phonon replicas of the latter optically inactive complexes. The semidark trions and negative biexcitons are distinguished. On the basis of their experimentally extracted and theoretically calculated g-factors, we identify three distinct families of emissions due to exciton complexes in WS,: bright, intravalley, and intervalley dark. The g-factors of the spin-split subbands in both the conduction and valence bands are also determined.
Klíčová slova
tungsten disulfide monolayer; exciton; trion; dark exciton; phonon replica; biexciton
Autoři
ZINKIEWITZ, M.; WOZNIAK, T.; KAZIMIERCZUK, T.; KAPUSCINSKI, P.; ORESZCZUK, K.; GRZESZCZYK, M.; BARTOŠ, M.; NOGAJEWSKI, K.; WATANABE, K.; TANIGUCHI, T.; FAUGERAS, C.; KOSSACKI, P.; POTEMSKI, M.; BABINSKI, A.; MOLAS, M.
Vydáno
24. 3. 2021
Nakladatel
American Chemical Society
Místo
WASHINGTON
ISSN
1530-6984
Periodikum
NANO LETTERS
Ročník
21
Číslo
6
Stát
Spojené státy americké
Strany od
2519
Strany do
2525
Strany počet
7
URL
https://pubs.acs.org/doi/10.1021/acs.nanolett.0c05021
Plný text v Digitální knihovně
http://hdl.handle.net/11012/202273
BibTex
@article{BUT172975, author="Malgorzata {Zinkiewitz} and Tomasz {Wozniak} and Tomasz {Kazimierczuk} and Piotr {Kapuscinski} and Kacper {Oreszczuk} and Magdalena {Grzeszczyk} and Miroslav {Bartoš} and Karol {Nogajewski} and Kenji {Watanabe} and Takashi {Taniguchi} and Clément {Faugeras} and Piotr {Kossacki} and Marek {Potemski} and Adam {Babinski} and Maciej {Molas}", title="Excitonic Complexes in n-Doped WS2 Monolayer", journal="NANO LETTERS", year="2021", volume="21", number="6", pages="2519--2525", doi="10.1021/acs.nanolett.0c05021", issn="1530-6984", url="https://pubs.acs.org/doi/10.1021/acs.nanolett.0c05021" }