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KEPIČ, P. LIŠKA, P. IDESOVÁ, B. CAHA, O. LIGMAJER, F. ŠIKOLA, T.
Originální název
Pulsed laser deposition of Sb2S3 films for phase-change tunable nanophotonics
Typ
článek v časopise ve Web of Science, Jimp
Jazyk
angličtina
Originální abstrakt
Non-volatile phase-change materials with large optical contrast are essential for future tunable nanophotonic applications. Antimony trisulfide (Sb2S3) has recently gained popularity in this field due to its low absorption in the visible spectral region. Although several Sb2S3 deposition techniques have been reported in the literature, none of them was optimized with respect to stoichiometry, lowest possible absorption, and large refractive index contrast (Delta n) upon the phase change. Here we present a comprehensive multi-parameter optimization of pulsed laser deposition of Sb2S3 towards this end. We correlate the specific deposition with the resulting compositional and optical properties and report parameters leading to films with extraordinary qualities (Delta n = 1.2 at 633 nm). Additionally, we suggest crystal orientations and vibrational modes associated with the largest change in the refractive index and propose them as useful large-scale indicators of the Sb2S3 switching contrast.
Klíčová slova
Sb2S3; tunable nanophotonics; phase-change materials
Autoři
KEPIČ, P.; LIŠKA, P.; IDESOVÁ, B.; CAHA, O.; LIGMAJER, F.; ŠIKOLA, T.
Vydáno
8. 1. 2024
Nakladatel
IOP Publishing Ltd
Místo
BRISTOL
ISSN
1367-2630
Periodikum
NEW JOURNAL OF PHYSICS
Ročník
26
Číslo
1
Stát
Spojené království Velké Británie a Severního Irska
Strany od
Strany do
8
Strany počet
URL
https://iopscience.iop.org/article/10.1088/1367-2630/ad1696
Plný text v Digitální knihovně
http://hdl.handle.net/11012/245215
BibTex
@article{BUT187206, author="Peter {Kepič} and Petr {Liška} and Beáta {Idesová} and Ondřej {Caha} and Filip {Ligmajer} and Tomáš {Šikola}", title="Pulsed laser deposition of Sb2S3 films for phase-change tunable nanophotonics", journal="NEW JOURNAL OF PHYSICS", year="2024", volume="26", number="1", pages="8", doi="10.1088/1367-2630/ad1696", issn="1367-2630", url="https://iopscience.iop.org/article/10.1088/1367-2630/ad1696" }