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VACULOVIČOVÁ, M. AKTHER, M. MAASKANT, P. BRABAZON, D. MACKA, M.
Original Title
Fibre coupled micro-light emitting diode array light source with integrated band-pass filter for fluorescence detection in miniaturised analytical systems
Type
journal article in Web of Science
Language
English
Original Abstract
In this work, a new type of miniaturized fibre-coupled solid-state light source is demonstrated as an excitation source for fluorescence detection in capillary electrophoresis. It is based on a parabolically shaped micro-light emitting diode (mu-LED) array with a custom band-pass optical interference filter (IF) deposited at the back of the LED substrate. The GaN mu-LED array consisted of 270 individual mu-LED elements with a peak emission at 470 nm, each about 14 mm in diameter and operated as a single unit. Light was extracted through the transparent substrate material, and coupled to an optical fibre (OF, 400 mm in diameter, numerical aperture NA = 0.37), to form an integrated mu-LED-IF-OF light source component. This packaged mu-LED-IF-OF light source emitted approximately 225 mu W of optical power at a bias current of 20 mA. The bandpass IF filter was designed to reduce undesirable LED light emissions in the wavelength range above 490 nm. Devices with and without IF were compared in terms of the optical power output, spectral characteristics as well as LOD values. While the IF consisted of only 7.5 pairs (15 layers) of SiO2/HfO2 layers, it resulted in an improvement of the baseline noise as well as the detection limit measured using fluorescein as test analyte, both by approximately one order of magnitude, with a LOD of 1 x 10(-8) mol L-1 obtained under optimised conditions. The mu-LED-IF-OF light source was then demonstrated for use in capillary electrophoresis with fluorimetric detection. The limits of detection obtained by this device were compared to those obtained with a commercial fibre coupled LED device.
Keywords
Micro-light emitting diode array; Light source; Optical fibre; Capillary electrophoresis; Fluorescence detection; Separations
Authors
VACULOVIČOVÁ, M.; AKTHER, M.; MAASKANT, P.; BRABAZON, D.; MACKA, M.
Released
29. 4. 2015
ISBN
0003-2670
Periodical
ANALYTICA CHIMICA ACTA
Year of study
871
Number
1
State
Kingdom of the Netherlands
Pages from
85
Pages to
92
Pages count
8
BibTex
@article{BUT145849, author="VACULOVIČOVÁ, M. and AKTHER, M. and MAASKANT, P. and BRABAZON, D. and MACKA, M.", title="Fibre coupled micro-light emitting diode array light source with integrated band-pass filter for fluorescence detection in miniaturised analytical systems", journal="ANALYTICA CHIMICA ACTA", year="2015", volume="871", number="1", pages="85--92", doi="10.1016/j.aca.2015.02.044", issn="0003-2670" }