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Liu, JJ. Jiang, SD. Neugebauer, P. van Slageren, J. Lan, YH. Wernsdorfer, W. Wang, BW. Gao, S.
Originální název
Magnetic and HFEPR Studies of Exchange Coupling in a Series of it mu-Cl Dicobalt Complexes
Typ
článek v časopise ve Web of Science, Jimp
Jazyk
angličtina
Originální abstrakt
We report three dinuclear cobalt(II) complexes, [Co(L)Cl-2](2) (L = bpy, mbpy, and dmpbt), that are bridged solely by chloride ions. High-field electron paramagnetic resonance and magnetometric measurements were applied to investigate the magnetic intramolecular Co-Co interactions. Simulation results based on the multispin model reveal that the complexes are weakly ferromagnetically coupled and that the isotropic exchange coupling constants differ slightly for the three complexes. Moreover, the competing effects of zero-field splitting and magnetic coupling on the temperature-dependent magnetic susceptibility were analyzed.
Klíčová slova
SINGLE-MOLECULE MAGNET; ELECTRON-PARAMAGNETIC-RESONANCE; TRANSITION-METAL-COMPLEXES; COBALT(II) COMPLEXES; WEAK FERROMAGNETISM; BRIDGE ANGLE; ANISOTROPY; LIGAND; CHAIN; DIMER
Autoři
Liu, JJ. ; Jiang, SD. ; Neugebauer, P. ; van Slageren, J. ; Lan, YH. ; Wernsdorfer, W. ; Wang, BW.; Gao, S.
Vydáno
6. 3. 2017
ISSN
0020-1669
Periodikum
Inorganic Chemistry
Ročník
56
Číslo
5
Stát
Spojené státy americké
Strany od
2417
Strany do
2425
Strany počet
9
BibTex
@article{BUT146446, author="Liu, JJ. and Jiang, SD. and Neugebauer, P. and van Slageren, J. and Lan, YH. and Wernsdorfer, W. and Wang, BW. and Gao, S.", title="Magnetic and HFEPR Studies of Exchange Coupling in a Series of it mu-Cl Dicobalt Complexes", journal="Inorganic Chemistry", year="2017", volume="56", number="5", pages="2417--2425", doi="10.1021/acs.inorgchem.6b02368", issn="0020-1669" }